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Neutron Scattering and Complementary Methods in Investations of Condensed Phase

autori
S. Urban, V. Domenici, J. Czub, M. Geppi, B. Gestblom, C.A. Veracini
anno
2003
tipo prodotto
Capitolo, parte o articolo in libro
lingua
inglese
casa editrice
Janusz Chrusciel
numero pagine
8
pagina iniziale
121
pagina finale
128
edizione
University of Podlasie Publishing House
ABSTRACT
Results of studies of 4-4'-di-n-heptylazoxybenzene (HAB) in the isotropic, nematic and smectic A phases are presented. Two experimental methods were applied: broad and dieletric spectroscopy (DS) and the nuclear magnetic resonance (NMR). The complex dielectric permittivity, epsilon*(w)= epsilon'(w)-iepsilon''(w), was measured in the frequency range 1 KHz - GHz. This allowed two main relaxation processes in all the phases studied to be separated: the low frequenciy, l.f., process connected with molecular reorientations aroung a short axes, and the high frequenc, h.f., process connected with rotations around the long axes. The measurement of 2H spin lattice relaxation times was carried out throughout the mesophase range of 10.0, 46.04 and 61.38 MHz. Using suitable theoretical models the principal components of the diffusion tensor, D// and D perpendicular, as well as the diffusion coefficients DR, relative to the internal rotation of the phenyl rings, were determined. The results of both studies are confronted and discussed.
schede autori
VERACINI CARLO ALBERTO